1. 上海勘察设计研究院有限公司,上海,200093
2. 上海环境岩土工程技术研究中心,上海,200093
纸质出版:2021
移动端阅览
陈展, 吴育林, 张刚. 上海市某大型再开发场地土壤重金属污染特征、评价及来源分析[J]. 水土保持通报, 2021,41(1):227-236.
Chen Zhan, Wu Yulin, Zhang Gang. Pollution Characteristics, Assessment, and Source Analysis of Soil Heavy Metals in Large-scale Redevelopment Site in Shanghai City[J]. Bulletin of Soiland Water Conservation, 2021, 41(1): 227-236.
陈展, 吴育林, 张刚. 上海市某大型再开发场地土壤重金属污染特征、评价及来源分析[J]. 水土保持通报, 2021,41(1):227-236. DOI: 10.13961/j.cnki.stbctb.2021.01.032.
Chen Zhan, Wu Yulin, Zhang Gang. Pollution Characteristics, Assessment, and Source Analysis of Soil Heavy Metals in Large-scale Redevelopment Site in Shanghai City[J]. Bulletin of Soiland Water Conservation, 2021, 41(1): 227-236. DOI: 10.13961/j.cnki.stbctb.2021.01.032.
[目的] 研究土壤中重金属污染与生态风险状况,为保障城市更新改造过程中土地的合理利用提供科学依据。[方法] 以上海市某大型再开发利用场地为研究对象,采集了102个点位的表层(0-0.5 m)和下层(1.5-2.0 m)土壤样品,测定10种重金属(As,Be,Cu,Pb,Ni,TI,Zn,Cd,Cr和Hg)浓度,采用地累积指数、内梅罗指数和潜在生态风险指数进行土壤重金属污染和生态风险评价,并进一步利用多元统计分析方法揭示土壤中重金属的来源情况。[结果] ①测试土壤中重金属均未超过《土壤环境质量建设用地土壤污染风险管控标准(试行)》(GB36600-2018)第二类用地风险筛选值,但6.9%,24.5%,25.5%,37.3%和63.7%的采样点土壤中As,Cu,Pb,Zn和Hg浓度超过土壤元素背景值,存在不同程度的累积现象。内梅罗指数评价结果表明研究区域土壤整体处于尚清洁到轻度污染状态,分别有11.8%和3.84%的表层区域与2.64%和0.63%的下层区域土壤呈中度污染和重度污染状态。②表层土壤综合潜在生态风险指数均值为89.91,处于中等风险水平,Hg为研究区域主要的生态风险因子。③土壤中Ni,Cr,Be和TI浓度主要受成土母质风化作用的自然源控制,Pb,Zn,Cu,As和Hg主要受交通运输源和历史农业活动源的影响,其中自然源对表层土壤中的As和下层土壤中Cu也有相当比例的贡献,而表层土壤中Hg更多受到除交通运输源以外的其他人类活动源影响。[结论] 后续土地利用过程应注重Hg的生态风险管控,并提高对外来交通源引起的重金属累积效应的关注。
[Objective] The heavy metal pollution characteristics and ecological risk for soil were studied to provide a scientific basis for the proper land use in the process of urban renewal.[Methods] Samples of topsoil (0-0.5 m) and subsoil (1.5-2.0 m) were collected from 102 point locations in a large-scale redevelopment site in Shanghai City
and the concentration levels of 10 heavy metals (As
Be
Cu
Pb
Ni
Ti
Zn
Cr
Cd
and Hg) were tested and measured. The heavy metal contamination and ecological risk were evaluated with geo-accumulation
Nemerow
and potential ecological risk indices. The sources of heavy metals were further identified and revealed by multivariate statistical analysis.[Results] ① The contents of the heavy metals in soil were lower than the type Ⅱ land soil risk screening values stipulated in the "Soil Environmental Quality-Risk Control Standard for Soil Contamination of Development Land
Pilot Version" (GB36600
2018)
but the contents of As
Cu
Pb
Zn
and Hg in soil from 6.9%
24.5%
25.5%
37.3%
and 63.7% sampling points exceed the background values of soil elements
which indicated different degrees of accumulation. The soil in the entire study area generally varies from clean to slightly polluted
with 11.8% and 3.84% of the topsoil and 2.64% and 0.63% of the subsoil moderately and heavily contaminated
respectively. ② The mean value of the comprehensive potential ecological risk index for topsoil was 89.91
representing a medium risk level. Hg in topsoil was the main ecological risk factor in the study area. ③ The concentrations of Ni
Cr
Be
and TI in the soil were mainly controlled by natural sources of weathering of the soil parent material. Pb
Zn
Cu
As
and Hg contents in soil were mostly affected by sources of transportation and historical agricultural production activities. Natural sources also contributed a considerable proportion to the contents of As in topsoil and Cu in subsoil as well as man-made sources. Hg in topsoil was more affected by other human activity sources than transportation sources.[Conclusion] During subsequent land use processes
more attention should be paid to the ecological risk control of Hg and the cumulative effect of heavy metals caused by external traffic sources.
范俊楠,郭丽,张明杰,等.湖北省重点区域及周边表层土壤重金属污染现状及评价[J].中国环境监测,2020,36(1):96-104.
熊佳,韩志伟,吴攀,等.独山锑冶炼厂周边土壤锑砷空间分布特征、污染评价及健康风险评估[J].环境科学学报,2020,40(2):655-664.
王洋洋,李方方,王笑阳,等.铅锌冶炼厂周边农田土壤重金属污染空间分布特征及风险评估[J].环境科学,2019,40(1):437-444.
Li Jingjing, Cui Jihua, Liu Gao, et al. Extensive study of potential harmful elements (Ag, As, Hg, Sb, and Se) in surface sediments of the Bohai Sea, China:Sources and environmental risks[J]. Environmental Pollution, 2016,219:432-439.
Jaffar S T A, Chen Longzhu, Younas H, et al. The extent of heavy metal pollution and their potential health risk in topsoils of the massively urbanized district of Shanghai[J]. Archives of Environmental Contamination and Toxicology, 2017,73(3):1-15.
Rajkumar H, Naik P K, Rishi M S. Evaluation of heavy metal contamination in soil using geochemical indexing approaches and chemometric techniques[J]. International Journal of Environmental Science and Technology, 2019,16(11):7467-7486.
刘庚,石瑛,田海金,等.某大型砷渣场地土壤As污染特征及生态风险评价[J].环境科学,2018,39(12):5639-5646.
张云芸,马瑾,魏海英,等.浙江省典型农田土壤重金属污染及生态风险评价[J].生态环境学报,2019,28(6):1233-1241.
Muller G. Index of geoaccumulation in sediments of the Rhine River[J]. Geojournal, 1969,2(3):108-118.
Hakanson L. An ecological risk index for aquatic pollution control. A sedimentological approach[J]. Water Research, 1980,14(8):975-1001.
徐争启,倪师军,庹先国,等.潜在生态危害指数法评价中重金属毒性系数计算[J].环境科学与技术,2008,31(2):112-115.
Kowalska J B, Mazurek R, Gasiorek M, et al. Pollution indices as useful tools for the comprehensive evaluation of the degree of soil contamination:A review[J]. Environmental Geochemistry and Health, 2018,40(6):2395-2420.
Xiong Bijing, Zhang Youchi, Nunes L M, et al. Critical comparison of soil pollution indices for assessing contamination with toxic metals[J]. Water, Air & Soil Pollution, 2015, 226(10):352.
王玉军,吴同亮,周东美,等.农田土壤重金属污染评价研究进展[J].农业环境科学学报,2017,36(12):2365-2378.
陈晓燕,范成五,瞿飞,等.土壤重金属污染评价方法概述[J].浙江农业科学,2017,58(10):1801-1804,1810.
郭彦海,孙许超,张士兵,等.上海某生活垃圾焚烧厂周边土壤重金属污染特征、来源分析及潜在生态风险评价[J].环境科学,2017,38(12):5262-5271.
张倩,陈宗娟,彭昌盛,等.大港工业区土壤重金属污染及生态风险评价[J].环境科学,2015,36(11):4232-4240.
徐晨,王沛芳,陈娟,等.望虞河西岸河网重金属污染特征及生态风险评价[J].环境科学,2019,40(11):4914-4923.
丁亚丽,廖敏,方至萍,等.新建铅蓄电池集聚区对周边土壤环境的影响:基于重金属空间特征[J].环境科学,2019,40(9):4244-4252.
纪冬丽,曾琬晴,张新波,等.天津近郊农田土壤重金属风险评价及空间主成分分析[J].环境化学,2019,38(9):1955-1965.
宁翠萍,李国琛,王颜红,等.细河流域农田土壤重金属污染评价及来源解析[J].农业环境科学学报,2017,36(3):487-495.
中华人民共和国环境保护部. HJ25.2-2014场地环境监测技术导则[S].北京:中国环境出版社,2015.
中华人民共和国环境保护总局. HJ/T166-2004土壤环境监测技术规范[S].北京:中国标准出版社,2004.
王云,汪雅谷,罗海林,等.上海市土壤环境背景值[M].北京:中国环境科学出版社,1992:37.
高瑞忠,张阿龙,张生,等.西北内陆盐湖盆地土壤重金属Cr, Hg, As空间分布特征及潜在生态风险评价[J].生态学报,2019,39(7):2532-2544.
Mazurek R, Kowalska J B, Gasiorek M, et al. Pollution indices as comprehensive tools for evaluation of the accumulation and provenance of potentially toxic elements in soils in Ojców National Park[J]. Journal of Geochemical Exploration, 2019,201:13-30.
宁增平,肖青相,蓝小龙,等.都柳江水系沉积物锑等重金属空间分布特征及生态风险[J].环境科学,2017,38(7):2784-2792.
徐志豪,吴健,王敏,等.典型复垦工业场地土壤垂直剖面重金属污染特征及潜在生态风险[J].水土保持通报,2019,39(2):43-47,55.
陈怡先,姜小三,王勇,等.基于GIS矿区土壤重金属生态环境及人体健康评价[J].环境科学学报,2018,38(4):1642-1652.
中华人民共和国生态环境部. GB36600-2018土壤环境质量建设用地土壤污染风险管控标准(试行)[S].北京:中国标准出版社,2018.
张连科,李海鹏,黄学敏,等.包头某铝厂周边土壤重金属的空间分布及来源解析[J].环境科学,2016,37(3):1139-1146.
黄润龙,管于华.数据统计分析-SPSS原理及应用[M].北京:高等教育出版社,2010:281-282.
刘敬勇,常向阳,涂湘林.重金属铊污染及防治对策研究进展[J].土壤,2007,39(4):528-535.
秦兵,陈代庚,任利民,等.成都盆地浅层土壤中砷来源的多元统计分析[J].安全與環境工程,2006,13(3):23-28.
李春芳,王菲,曹文涛,等.龙口市污水灌溉区农田重金属来源、空间分布及污染评价[J].环境科学,2017,38(3):1018-1027.
白一茹,张兴,赵云鹏,等.基于GIS和受体模型的枸杞地土壤重金属空间分布特征及来源解析[J].环境科学,2019,40(6):2885-2894.
Han Lanfang, Gao Bo, Hao Hong, et al. Lead contamination in sediments in the past 20 years:A challenge for China[J]. Science of the Total Environment, 2018,640/641:746-756.
邓霞,孙慧兰,杨余辉,等.伊宁市土壤中重金属污染评价及来源解析研究[J].环境污染与防治,2020,42(2):223-226,237.
孙厚云,吴丁丁,毛启贵,等.新疆东天山某铜矿区土壤重金属污染与生态风险评价[J].环境化学,2019,38(12):2690-2699.
冯新斌,陈玖斌,付学吾,等.汞的环境地球化学研究进展[J].矿物岩石地球化学通报,2013,32(5):503-530.
王立辉,邹正禹,张翔宇,等.土壤中汞的来源及土壤汞污染修复技术概述[J].现代化工,2015,35(5):43-47.
卢光华,岳昌盛,彭犇,等.汞污染土壤修复技术的研究进展[J].工程科学学报,2017,39(1):1-12.
0
浏览量
939
下载量
8
CSCD
关联资源
相关文章
相关作者
相关机构
京公网安备11010802024621